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A relationship between three-dimensional surface hydration structures and force distribution measured by atomic force microscopy
https://doi.org/10.24517/00009201
https://doi.org/10.24517/000092015168b386-9a99-4aba-b0c6-80e2e524a993
名前 / ファイル | ライセンス | アクション |
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TE-PR-FUKUMA-T-7334.pdf (469.4 kB)
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Item type | 学術雑誌論文 / Journal Article(1) | |||||
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公開日 | 2017-10-03 | |||||
タイトル | ||||||
タイトル | A relationship between three-dimensional surface hydration structures and force distribution measured by atomic force microscopy | |||||
言語 | ||||||
言語 | eng | |||||
資源タイプ | ||||||
資源タイプ識別子 | http://purl.org/coar/resource_type/c_6501 | |||||
資源タイプ | journal article | |||||
ID登録 | ||||||
ID登録 | 10.24517/00009201 | |||||
ID登録タイプ | JaLC | |||||
著者 |
Miyazawa, Keisuke
× Miyazawa, Keisuke× Kobayashi, Naritaka× Watkins, Matthew× Shluger, Alexander L.× Amano, Ken-ichi× Fukuma, Takeshi |
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著者別表示 |
福間, 剛士
× 福間, 剛士 |
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書誌情報 |
Nanoscale 巻 8, 号 13, p. 7334-7342, 発行日 2016-04-07 |
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ISSN | ||||||
収録物識別子タイプ | ISSN | |||||
収録物識別子 | 2040-3364 | |||||
DOI | ||||||
関連タイプ | isVersionOf | |||||
識別子タイプ | DOI | |||||
関連識別子 | 10.1039/c5nr08092d | |||||
出版者 | ||||||
出版者 | Royal Society of Chemistry | |||||
抄録 | ||||||
内容記述タイプ | Abstract | |||||
内容記述 | Hydration plays important roles in various solid-liquid interfacial phenomena. Very recently, three-dimensional scanning force microscopy (3D-SFM) has been proposed as a tool to visualise solvated surfaces and their hydration structures with lateral and vertical (sub) molecular resolution. However, the relationship between the 3D force map obtained and the equilibrium water density, ρ(r), distribution above the surface remains an open question. Here, we investigate this relationship at an interface of an inorganic mineral, fluorite, and water. The force maps measured in pure water are directly compared to force maps generated using the solvent tip approximation (STA) model and from explicit molecular dynamics simulations. The results show that the simulated STA force map describes the major features of the experimentally obtained force image. The agreement between the STA data and the experiment establishes the correspondence between the water density used as an input to the STA model and the experimental hydration structure and thus provides a tool to bridge the experimental force data and atomistic solvation structures. Further applications of this method should improve the accuracy and reliability of both interpretation of 3D-SFM force maps and atomistic simulations in a wide range of solid-liquid interfacial phenomena. © The Royal Society of Chemistry 2016. | |||||
内容記述 | ||||||
内容記述タイプ | Other | |||||
内容記述 | Embargo Period 12 months | |||||
著者版フラグ | ||||||
出版タイプ | AM | |||||
出版タイプResource | http://purl.org/coar/version/c_ab4af688f83e57aa |